Unfortunately, you will be unable to accomplish this in LabVIEW. This operation is not supported by the data acquisition driver. NI-DAQ will generate an error when trying to configure port C as two 4-bit ports. While NI-DAQ does not support this function, it is possible to use register-level programming. Application Note 131 includes sample register level programming code that will accomplish this task.
Application Note 131: Digital I/O Applications
http://zone.ni.com/devzone/conceptd.nsf/2d17d611efb58b22862567a9006ffe76/467ed254f3a30b1286256a6f00720951?OpenDocument
Regards,
Justin Britten
Applications Engineer
National Instruments